环境光/电催化

1. CO₂的捕集和光/电催化转化：尤其聚焦于实际环境中的CO₂（如空气、燃烧尾气）的直接转化利用，即实现对于低浓度CO₂的富集和在有氧条件下的选择性还原，同时也结合氮循环过程（硝酸盐和氨的转化）通过碳-氮偶联实现CO₂向高附加值化学品的转化。

2. 气/液界面上的协同光催化反应：光催化利用太阳光作为反应动力来源，在反应装置的搭建上具备高度的灵活性，不受空间和场地的限制。由此构建漂浮的光催化反应器件，可以实现气相还原反应（CO₂还原，O₂还原生成H₂O₂，NO_x去除等）和液相氧化反应（有毒难降解污染物的去除）的协同进行，构建可应用于开放水域的水-气净化装置。

3. 原位红外光谱系统的搭建和方法学发展：通过发展契合表面反应时间尺度（毫秒~秒）、多检测模式的红外光谱仪器和方法学，揭示光/电催化反应过程的微观机制。

1. 国家级青年人才, 2019.2-2022.2, 主持 

2. 中科院化学所创新培育项目，"CO₂深度还原机理的快速扫描红外光谱研究"，2020.1-2023.12，主持

3. 基金委面上项目，"基于新型电子/质子传递膜的双功能的光催化降解污染物体系"，No.22076193, 2021.1-2024.12，主持

4. 国家重点研发计划"变革性技术关键科学问题"，"面向地外原位资源利用技术的人工光合成关键材料与系统研究"，No.2020YFA0710303, 2020.12-2025.11，课题骨干

5. 中国科学院稳定支持基础研究领域青年团队计划， "高效光解水中的科学问题-光解水过程全时空域原位动态成像研究"，No.YSBR-004, 2021.6-2026.6，课题骨干

6. 基金委优秀青年基金项目，"环境光催化"，No.22222609，2023.1-2025.12，主持

7. 基金委创新研究群体项目，"污染物光催化降解和界面光化学转化"，No.22321004， 2024.1-2028.12，课题骨干

26. Yangfan Li(李杨凡), Xingmiao Huang, Boyang Zhang, Chuncheng Chen, Hua Sheng* and Jincai Zhao, "Mixed CO Adsorption Modes Induced by Lattice Strain to Facilitate C-C Coupling during Electrochemical CO Reduction", Appl. Catal. B-Environ. Energy, 2025, 361, 124627.

25. Wanyi Zhang^#(张晚依), Chaoyuan Deng^#, Wei Wang*(王伟), Hua Sheng* and Jincai Zhao, "Achieving Almost 100% Selectivity in Photocatalytic CO₂ Reduction to Methane via In-situ Atmosphere Regulation Strategy", Adv. Mater. 2024, 36(35), 2405825.

24. Reshalaiti Hailili*(热沙来提•海里里), Zelong Li, Xu Lu, Hua Sheng*, Detlef W. Bahnemann and Jincai Zhao, "Ultrathin Defective Heterojunction for Visible Light NO Removal: Correlation between Microstructure and Reaction Mechanism", Environ. Sci.-Nano, 2024, 11(8), 3301-3316. (Inside Cover)

23. Yangen Xie(谢杨恩), Min Wang, Qiang Huang, Qing Huang, Bo Sheng, Wenjing Song, Hua Sheng* and Jincai Zhao, "A Floatable Photocatalyst to Synergistically Promote CO₂ Reduction and Water Oxidation by Creating Oriented Charge Separation across a Tri-phase Interface", Energy Environ. Sci. 2024, 17(7), 4725-4734.

22. Baipeng Yin, Can Wang, Shijie Xie, Jianmin Gu, Hua Sheng*, De-Xian Wang*, Jiannian Yao and Chuang Zhang*, "Regulating Spin Density Using TEMPOL Molecules for Enhanced CO₂-to-Ethylene Conversion by HKUST-1 Framework Derived Electrocatalysts", Angew. Chem. Int. Ed. 2024, 63(29), e202405873.

21. Xingmiao Huang(黄星妙), Yangfan Li, Shijie Xie*(谢士杰), Qi Zhao, Boyang Zhang, Zhiyong Zhang, Hua Sheng* and Jincai Zhao, "The Tandem Nitrate and CO₂ Reduction for Urea Electrosynthesis: Role of Surface N-Intermediates in CO₂ Capture and Activation", Angew. Chem. Int. Ed. 2024, 63(24), e202403980.

20. Qing Huang(黄庆) and Hua Sheng*, "Magnetic-Field-Induced Spin Regulation in Electrocatalytic Reactions", Chem. Eur. J. 2024, 30(17), e202400352. (Invited Review)

19. Wei Wang^#(王伟), Wanyi Zhang^#(张晚依), Chaoyuan Deng, Hua Sheng* and Jincai Zhao, "Accelerated Photocatalytic Carbon Dioxide Reduction and Water Oxidation under Spatial Synergy", Angew. Chem. Int. Ed. 2024, 63(7), e202317969.

18. Bo Sheng(盛波), Yangen Xie, Qi Zhao, Hua Sheng* and Jincai Zhao, "Proton Reservoir in Polymer Photocatalysts for the Superior H₂O₂ Photosynthesis", Energy Environ. Sci. 2023, 16(10), 4612-4619.

17. Zhong-Ting Hu^#, Yan-Fei Fei^#, Qiong-Yu Wang, Qi Zhao, Siew-Leng Loo, Mian Hu, Yonghe Li, Yujie Song, Jie-Xin Wang, Zhi-Gang Shen, Hua Sheng*, Jiade Wang* and Jincai Zhao, "Catalytic Disinfection: Quasi-Dynamically Monitoring Bacteria Sterilization Based on CuNPs/ZnIn₂S₄ Disinfectants and in-situ CuNPs Regeneration", Appl. Catal. B-Environ. 2023, 337, 122995.

16. Qing Huang^#(黄庆), Shijie Xie^#(谢士杰), Jinjie Hao, Zijing Ding*, Chuang Zhang*, Hua Sheng* and Jincai Zhao, "Spin-Enhanced O-H Cleavage in Electrochemical Water Oxidation", Angew. Chem. Int. Ed. 2023, 62(20), e202300469. (Hot Paper)

15. Yangfan Li^#(李杨凡), Shijie Xie^#(谢士杰), Xingmiao Huang, Wenjing Song, Chuncheng Chen, Hua Sheng* and Jincai Zhao, "Spectating the Proton Migration on Catalyst with Noninnocent Ligand in Aqueous Electrochemical CO₂ Reduction", Appl. Catal. B-Environ. 2023, 329, 122542.

14. Shijie Xie^#(谢士杰), Chaoyuan Deng^#, Qing Huang, Chuang Zhang*, Chuncheng Chen, Jincai Zhao* and Hua Sheng*, "Facilitated Photocatalytic CO₂ Reduction in Aerobic Environment on a Copper-Porphyrin Metal-Organic Framework", Angew. Chem. Int. Ed. 2023, 62(10), e202216717.

Introducing...Hua Sheng, Angew. Chem. Int. Ed. 2023, 62(13), e202301138. 

12. Jinjie Hao, Shijie Xie, Qing Huang, Zijing Ding, Hua Sheng*, Chuang Zhang* and Jiannian Yao, "Spin-Enhanced C-C Coupling in CO₂ Electroreduction with Oxide-Derived Copper", CCS Chem. 2023, 5(9), 2046-2058.

13. Bo Sheng^#(盛波), Chaoyuan Deng^#, Yangfan Li, Shijie Xie, Zhaohui Wang*, Hua Sheng* and Jincai Zhao, "In-Situ Hydroxylation of Single-Atom Iron Catalyst for Preferential ¹O₂ Production from H₂O₂", ACS Catal. 2022, 12(23), 14679-14688.

11. Reshalaiti Hailili*(热沙来提•海里里), Hongwei Ji, Kaiwen Wang, Xing'an Dong, Chuncheng Chen, Hua Sheng*, Detlef W. Bahnemann* and Jincai Zhao, "ZnO with Controllable Oxygen Vacancies for Photocatalytic Nitrogen Oxide Removal", ACS Catal. 2022, 12(16), 10004-10017.

10. Shijie Xie^#(谢士杰), Yangfan Li^#(李杨凡), Bo Sheng, Wanyi Zhang, Wei Wang, Chuncheng Chen, Jikun Li*, Hua Sheng* and Jincai Zhao, "Self-Reconstruction of Paddle-Wheel Copper-Node to Facilitate the Photocatalytic CO₂ Reduction to Ethane", Appl. Catal. B-Environ. 2022, 310, 121320.

9. Reshalaiti Hailili^#(热沙来提•海里里), Zhi-Qiang Wang^#, Hongwei Ji, Chuncheng Chen, Xue-Qing Gong*, Hua Sheng* and Jincai Zhao, "Mechanistic Insights into the Photocatalytic Reduction of Nitric Oxide to Nitrogen on Oxygen-Deficient Quasi-Two-Dimensional Bismuth-Based Perovskites", Environ. Sci.-Nano 2022, 9(4), 1453-1465.

8. Wei Wang(王伟), Chaoyuan Deng, Shijie Xie, Yangfan Li, Wanyi Zhang, Hua Sheng*, Chuncheng Chen and Jincai Zhao, "Photocatalytic C-C Coupling from Carbon Dioxide Reduction on Copper Oxide with Mixed-Valence Copper(I)/Copper(II)", J. Am. Chem. Soc. 2021, 143(7), 2984-2993. 

7. Hongna Zhang, Yangfan Li, Jinzhao Wang, Ningning Wu, Hua Sheng*, Chuncheng Chen* and Jincai Zhao, "An Unprecedent Hydride Transfer Pathway for Selective Photocatalytic Reduction of CO₂ to Formic Acid on TiO₂", Appl. Catal. B-Environ. 2021, 284, 119692. 

6. Jose A. Corgejo^#, Hua Sheng^#, Eran Edri^#, Caroline M. Ajo-Franklin* and Heinz Frei*, "Nanoscale Membranes that Chemically Isolate and Electronically Wire Up the Abiotic/Biotic Interface", Nat. Commun. 2018, 9, 2263.

5. Hua Sheng, Myoung Hwan Oh, Wojciech T. Osowiecki, Wooyul Kim, A. Paul Alivisatos and Heinz Frei*, "Carbon Dioxide Dimer Radical Anion as Surface Intermediate of Photoinduced CO₂ Reduction at Aqueous Cu and CdSe Nanoparticle Catalysts by Rapid-Scan FT-IR Spectroscopy", J. Am. Chem. Soc. 2018, 140(12), 4363-4371.

Highlighted: "Dimers on the Way", by Davide Esposito, Nat. Catal. 2018, 1, 234.

4. Hua Sheng and Heinz Frei*, "Direct Observation by Rapid-Scan FT-IR Spectroscopy of Two-Electron-Reduced Intermediate of Tetraza Catalyst [Co^IIN₄H(MeCN)]²⁺ Converting CO₂ to CO", J. Am. Chem. Soc. 2016, 138(31), 9959-9967.

3. Hua Sheng, Hongna Zhang, Wenjing Song, Hongwei Ji, Wanhong Ma, Chuncheng Chen* and Jincai Zhao, "Activation of Water in Titanium Dioxide Photocatalysis by Formation of Surface Hydrogen Bonds: An In Situ IR Spectroscopy Study", Angew. Chem. Int. Ed. 2015, 54(20), 5905-5909.

2. Hua Sheng, Hongwei Ji, Wanhong Ma, Chuncheng Chen* and Jincai Zhao, "Direct Four-Electron Reduction of O₂ to H₂O on TiO₂ surface by Pendant Proton Relay", Angew. Chem. Int. Ed. 2013, 52(7), 9686-9690.

1. Hua Sheng, Qin Li, Wanhong Ma, Hongwei Ji, Chuncheng Chen* and Jincai Zhao, "Photocatalytic Degradation of Organic Pollutants on Surface Anionized TiO₂: Common Effect of Anions for High Hole-Availability by Water", Appl. Catal. B-Environ. 2013, 138, 212-218.